I'd think FFVIII's OST was the best, because of all the OSTs from FF, VIIIs was the most connected, most focused. The tracks seemed to follow a theme or a mood. None of them felt out of place... That's also why it's my favourite OST..
I'd say FFIX isn't bad because its got great tracks, but as a collective, the music is all over the place - but this was intended because FFIX was paying homage to the entire series at the same time.
VI is also another good one, but only if it was redone with a better synthesizer or orchestra
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